Dynamical Structure Factor in Cu Benzoate and other spin-1/2 antiferromagnetic chains

Recent experiments of the quasi-one-dimensional spin-1/2 antiferromagnet Copper Benzoate established the existence of a magnetic field induced gap. The observed neutron scattering intensity exhibits resolution limited peaks at both the antiferromagnetic wave number and at incommensurate wave numbers related to the applied magnetic field. We determine the ratio of spectral weights of these peaks within the framework of a low-energy effective field theory description of the problem.Comment: 5 pages, 3figure

Field-induced gap in the spin-1/2 antiferromagnetic Heisenberg chain: A density matrix renormalization group study

We study the spin-1/2 antiferromagnetic Heisenberg chain in both uniform and (perpendicular) staggered magnetic fields using the density-matrix renormalization-group method. This model has been shown earlier to describe the physics of the copper benzoate materials in magnetic field. In the present work, we extend the study to more general case for a systematic investigation of the field-induced gap and related properties of the spin-1/2 antiferromagnetic Heisenberg chain. In particular, we explore the high magnetic field regime where interesting behaviors in the field-induced gap, magnetization, and spin correlation functions are found. Careful examination of the low energy properties and magnetization reveals interesting competing effects of the staggered and uniform fields. The incommensurate behavior in the spin correlation functions is demonstrated and discussed in detail. The present work reproduces earlier results in good agreement with experimental data on copper benzoate and predicts new interesting field-induced features at very high magnetic field.Comment: 8 pages, 6 figure

Spectral functions of the Falicov-Kimball model with electronic ferroelectricity

We calculate the angular resolved photoemission spectrum of the Falicov-Kimball model with electronic ferroelectricity where $d$- and $f$-electrons have different hoppings. In mix-valence regimes, the presence of strong scattering processes between $d$-$f$ excitons and a hole, created by emission of an electron, leads to the formation of pseudospin polarons and novel electronic structures with bandwidth scaling with that of $d$-$f$ excitons. Especially, in the two-dimensional case, we find that flat regions exist near the bottom of the quasiparticle band in a wide range of the $d$- and $f$-level energy difference.Comment: 5 pages, 5 figure

Correlation Amplitudes for the spin-1/2 XXZ chain in a magnetic field

We present accurate numerical estimates for the correlation amplitudes of leading and main subleading terms of the two- and four-spin correlation functions in the one-dimensional spin-1/2 XXZ model under a magnetic field. These data are obtained by fitting the correlation functions, computed numerically with the density-matrix renormalization-group method, to the corresponding correlation functions in the low-energy effective theory. For this purpose we have developed the Abelian bosonization approach to the spin chain under the open boundary conditions. We use the numerical data of the correlation amplitudes to quantitatively estimate spin gaps induced by a transverse staggered field and by exchange anisotropy.Comment: 18 pages, 6 figures, 1 tabl

Coupled S=1/2S=1/2 Heisenberg antiferromagnetic chains in an effective staggered field

We present a systematic study of coupled $S=1/2$ Heisenberg antiferromagnetic chains in an effective staggered field. We investigate several effects of the staggered field in the {\em higher} ({\em two or three}) {\em dimensional} spin system analytically. In particular, in the case where the staggered field and the inter-chain interaction compete with each other, we predict, using mean-field theory, a characteristic phase transition. The spin-wave theory predicts that the behavior of the gaps induced by the staggered field is different between the competitive case and the non-competitive case. When the inter-chain interactions are sufficiently weak, we can improve the mean-field phase diagram by using chain mean-field theory and the analytical results of field theories. The ordered phase region predicted by the chain mean-field theory is substantially smaller than that by the mean-field theory.Comment: 13pages, 12figures, to be published in PR

Two-spinon dynamic structure factor of the one-dimensional S=1/2 Heisenberg antiferromagnet

The exact expression derived by Bougourzi, Couture, and Kacir for the 2-spinon contribution to the dynamic spin structure factor $S_{zz}(q,\omega)$ of he one-dimensional $S$=1/2 Heisenberg antiferromagnet at $T=0$ is evaluated for direct comparison with finite-chain transition rates ($N\leq 28$) and an approximate analytical result previously inferred from finite-$N$ data, sum rules, and Bethe-ansatz calculations. The 2-spinon excitations account for 72.89% of the total intensity in $S_{zz}(q,\omega)$. The singularity structure of the exact result is determined analytically and its spectral-weight distribution evaluated numerically over the entire range of the 2-spinon continuum. The leading singularities of the frequency-dependent spin autocorrelation function, static spin structure factor, and $q$-dependent susceptibility are determined via sum rules.Comment: 6 pages (RevTex) and 5 figures (Postscript

High-field magnetization study of the S = 1/2 antiferromagnetic Heisenberg chain [PM Cu(NO3_3)2_2(H2_2O)2_2]n_n with a field-induced gap

We present a high-field magnetization study of the $S$ = 1/2 antiferromagnetic Heisenberg chain [PM Cu(NO$_3$)$_2$(H$_2$O)$_2$]$_n$. For this material, as result of the Dzyaloshinskii-Moriya interaction and a staggered $g$ tensor, the ground state is characterized by an anisotropic field-induced spin excitation gap and a staggered magnetization. Our data reveal the qualitatively different behavior in the directions of maximum and zero spin excitation gap. The data are analyzed via exact diagonalization of a linear spin chain with up to 20 sites and on basis of the Bethe ansatz equations, respectively. For both directions we find very good agreement between experimental data and theoretical calculations. We extract the magnetic coupling strength $J/k_B$ along the chain direction to 36.3(5) K and determine the field dependence of the staggered magnetization component $m_s$.Comment: 5 pages, 2 figures (minor changes to manuscript and figures

Sr2V3O9 and Ba2V3O9: quasi one-dimensional spin-systems with an anomalous low temperature susceptibility

The magnetic behaviour of the low-dimensional Vanadium-oxides Sr2V3O9 and Ba2V3O9 was investigated by means of magnetic susceptibility and specific heat measurements. In both compounds, the results can be very well described by an S=1/2 Heisenberg antiferromagnetic chain with an intrachain exchange of J = 82 K and J = 94 K in Sr2V3O9 and Ba2V3O9, respectively. In Sr2V3O9, antiferromagnetic ordering at T_N = 5.3 K indicate a weak interchain exchange of the order of J_perp ~ 2 K. In contrast, no evidence for magnetic order was found in Ba2V3O9 down to 0.5 K, pointing to an even smaller interchain coupling. In both compounds, we observe a pronounced Curie-like increase of the susceptibility below 30 K, which we tentatively attribute to a staggered field effect induced by the applied magnetic field. Results of LDA calculations support the quasi one-dimensional character and indicate that in Sr2V3O9, the magnetic chain is perpendicular to the structural one with the magnetic exchange being transferred through VO4 tetrahedra.Comment: Submitted to Phy. Rev.

Critical properties of 1-D spin 1/2 antiferromagnetic Heisenberg model

We discuss numerical results for the 1-D spin 1/2 antiferromagnetic Heisenberg model with next-to-nearest neighbour coupling and in the presence of an uniform magnetic field. The model develops zero frequency excitations at field dependent soft mode momenta. We compute critical quantities from finite size dependence of static structure factors.Comment: talk given by H. Kr{\"o}ger at Heraeus Seminar Theory of Spin Lattices and Lattice Gauge Models, Bad Honnef (1996), 20 pages, LaTeX + 18 figures, P

Quantum criticalities in a two-leg antiferromagnetic S=1/2 ladder induced by a staggered magnetic field

We study a two-leg antiferromagnetic spin-1/2 ladder in the presence of a staggered magnetic field. We consider two parameter regimes: strong (weak) coupling along the legs and weak (strong) coupling along the rungs. In both cases, the staggered field drives the Haldane spin-liquid phase of the ladder towards a Gaussian quantum criticality. In a generalized spin ladder with a non-Haldane, spontaneously dimerized phase, the staggered magnetic field induces an Ising quantum critical regime. In the vicinity of the critical lines, we derive low-energy effective field theories and use these descriptions to determine the dynamical response functions, the staggered spin susceptibility and the string order parameter.Comment: 29 pages of revtex, 10 figure